Izvestiya of Saratov University.

Physics

ISSN 1817-3020 (Print)
ISSN 2542-193X (Online)


For citation:

Isaeva E. A., Isaeva A. A., Zimnyakov D. A. Referenceless Low-Coherence Reflectometry of Random Media under Wide-Band Spectral Selection of Scattered Probe Light. Izvestiya of Saratov University. Physics , 2019, vol. 19, iss. 4, pp. 270-278. DOI: 10.18500/1817-3020-2019-19-4-270-278

This is an open access article distributed under the terms of Creative Commons Attribution 4.0 International License (CC-BY 4.0).
Published online: 
02.12.2019
Full text:
(downloads: 359)
Language: 
Russian
UDC: 
535.37+681.785.57

Referenceless Low-Coherence Reflectometry of Random Media under Wide-Band Spectral Selection of Scattered Probe Light

Autors: 
Isaeva Elena Andreevna, Yuri Gagarin State Technical University of Saratov
Isaeva Anna Andreevna, Yuri Gagarin State Technical University of Saratov
Zimnyakov Dmitry Aleksandrovich, Yuri Gagarin State Technical University of Saratov
Abstract: 

Background and Objectives: The optical probes of randomly inhomogeneous media, based on analysis of the statistical parameters of the scattered light intensity, are sensitive to optical, structural, and transport parameters of the medium. A promising approach among the low-coherence optical methods is an approach in which the medium is considered as a multi-beam interferometer with randomly distributed values of the path difference of the interfering beams (partial waves). It is interesting to verify the potential of the referenceless low coherence reflectometry using a detection system with the low spectral selectivity (for example, a portable spectrometer with the spectral resolution of about 1 nm). On the one hand, the study of the dynamics and spectral features of fluorescence caused by the structural properties of the media makes it possible to explore more deeply the fundamental processes of conversion, transfer and amplification of radiation in heterogeneous micro- and nanostructured systems. On the other hand, such study will expand the potential of the existing low-coherence techniques. The aim of this work was a statistical analysis of stochastic interference fields generated by the strongly scattering fluorescent media using the reference-free path length low-coherence reflectometry under the condition of low spectral selectivity of the detection system. Materials and Methods: The investigation of the stochastic interference of the fluorescence radiation scattered by the dye-doped random medium using reference-free path length reflectometry under the condition of low spectral selectivity of the detection system was carried out. A water solution of Rhodamine 6G was used as the dye. Strongly scattering media were composed by close-packed titanium dioxide particles. The width of the spectral window was about 1 nm. The probability distributions of the optical path length of partial components and their differences were evaluated by using Monte–Carlo simulation with certain parameters of the modeled medium (the refractive index, the reduced scattering coefficient and the absorption coefficient). Results: The strong dispersion of the oscillation index of fluorescent radiation was observed. Such significant non-monotonic behavior of the oscillation index can be interpreted in terms of the influence of the absorption and scattering of fluorescent radiation in the probed medium on the probability density of path difference of the partial components of fluorescent radiation. In particular, the maximum of the oscillation index observed at the high-frequency boundary of the analyzed spectral range is presumably caused by the optical absorbance of Rhodamine solution at the long-wavelength region. A sharp decrease of the oscillation index curve in the spectral range from 580 nm to 630 nm, which correlates with a significant increase in the fluorescence intensity in this interval, is presumably caused by the effect of spontaneous amplification of fluorescence radiation. The obtained data correlate with previously reported data for the case of narrow spectral selection with the spectral window about 0.05 nm. Conclusion: It was shown that the reference-free path low-coherence reflectometry based on the statistical analysis of spatial fluctuations of the radiation intensity can be implemented using spectrometric systems with relatively low resolution (with the spectral window width about 1 nm). Such studies can be considered as the physical basis for creating new approaches and improving the existing ones to fluorescence diagnostics of the randomly inhomogeneous media in the biomedicine and material science.

Reference: 
  1. Brunel L., Brun A., Snabre P., Cipelletti L. Adaptive speckle imaging interferometry: a new technique for the analysis of microstructure dynamics, drying processes and coating formation. Optics Express, 2007, vol. 15, no. 23, pp. 15250–15259. DOI: https://doi.org/10.1364/OE.15.015250
  2. Liu B., Brezinski M. E. Theoretical and practical considerations on detection performance of time domain, Fourier domain, and swept source optical coherence tomography. J. Biomed. Opt., 2007, vol. 12, iss. 4, pp. 044007–0440011. DOI: https://doi.org/10.1117/1.2753410
  3. Zakharov P., Cardinaux F., Scheffold F. Multispeckle diffusing-wave spectroscopy with a single-mode detection scheme. Phys. Rev. E Stat. Nonlin. Soft Matter Phys., 2006, vol. 73, iss. 1, pp. 011413–011416. DOI: https://doi.org/10.1103/PhysRevE.73.011413
  4.  Proskurin S. G., Kuskova N. A., Avsievich T. I. Optical Doppler Methods for the Measurements of Flow Velocities of Biological Liquids. Izv. Saratov Univ. (N. S.), Ser. Physics, 2017, vol. 17, iss. 4, pp. 269–280 (in Russian). DOI: https://doi.org/10.18500/1817-3020-2017-17-4-269-280
  5. Huang D., Swanson E. A., Lin C. P., Schuman J. S., Stinson W. G., Chang W., Hee M. R., Flotte T., Gregory K., Puliafi to C. A., Fujimoto J. G. Optical coherence tomography. Science, 1991, vol. 5035, iss. 254, pp. 1178–1181 DOI: https://doi.org/10.1126/science.1957169
  6. Fujimoto J. G., Brezinski M. E., Tearney G. J., Boppart S. A., Bouma B., Hee M. R., Southern J. F., Swanson E. A. Optical biopsy and imaging using optical coherence tomography. Nat. Med, 1995, vol. 1, pp. 970–972.
  7. Narayan R. J. Monitoring and Evaluation of Biomaterials and Their Performance in Vivo. Amsterdam, Woodhead Publishing. 2017. 224 p.
  8. Shirazi M. F., Jeon M., Kim J. Structural Analysis of Polymer Composites Using Spectral Domain Optical Coherence Tomography. Sensors (Basel), 2017, vol. 5, iss.17, pp. 1155. DOI: https://doi.org/10.3390/s17051155
  9. Ulyanov S. S., Ulianova O. V., Zaitsev S. S., Khizhnyakova M. A., Saltykov Yu. V., Filonova N. N., Subbotina I. A., Lyapina A. M., Feodorova V. A. Study of Statistical Characteristics of GB-speckles, Forming at Scattering of Light on Virtual Structures of Nucleotide Gene Sequences of Enterobacteria. Izv. Saratov Univ. (N. S.), Ser. Physics, 2018, vol. 18, iss. 2, pp. 123–137 (in Russian). DOI: https://doi.org/10.18500/1817-3020-2018-18-2-123-137
  10. Durian D. J., Weitz D. A., Pine D. J. Dynamics and coarsening in three-dimensional foams. J. Phys. Condens. Matter., 1990, vol. 2, pp. SA433–SA436. DOI: https://doi.org/10.1088/0953-8984/2/S/069
  11. Isaeva A. A., Isaeva E. A. Spatially resolved speckle correlometry in application to media structure characterization. IEEE, Laser Optics, International Conference, 2014, vol. 6886501, pp. 501214. DOI: https://doi.org/10.1109/LO.2014.6886501  
  12. Zimnyakov D. A., Isaeva A. A., Isaeva E. A., Ushakova O.V. Speckle-correlation analysis of the dynamic scatterers in temperature-governed gelation. Proc. SPIE., 2016, vol. 9917, pp. 99172E–99178E. DOI: https://doi.org/10.1117/12.2229822
  13. Zimnyakov D. A., Sadovoi A. V., Vilenskii M. A., Zakharov P. V., Myllylä R. Critical behavior of phase interfaces in porous media: Analysis of scaling properties with the use of noncoherent and coherent light. JETP, 2009, vol. 108, no. 2, pp. 311–325. DOI: https://doi.org/10.1134/S1063776109020149
  14. Zimnyakov D. A., Yuvchenko S. A., Pavlova M. V., Alonova M. V. Reference-free path length interferometry of random media with the intensity moments analysis. Optics Express, 2017, vol. 25, iss. 13, pp. 13953–13972. DOI: https://doi.org/10.1364/OE.25.013953
  15. Wiersma D. S., Lagendijk A. Light diffusion with gain and random lasers. Phys. Rev. E, 1996, vol. 54, iss. 4, pp. 4256–4265.
  16. Van der Molen K. L., Mosk A. P., Lagendijk A. Quantitative analysis of several random lasers. Opt. Commun., 2007, vol. 278, pp. 110–113. DOI: https://doi.org/10.1016/j.optcom.2007.05.047
  17. El-Dardiry R. G., Lagendijk A. Tuning random lasers by engineered absorption. App. Phys. Lett., 2011, vol. 98, iss. 16, pp. 161106–08. DOI: https://doi.org/10.1063/1.3571452
  18. Colodrero S., Calvo M. E., Miguez H. Photon management in dye sensitized solar cells. Available at: https://www.researchgate.net/publication/221907408_Photon_Management_in_... (accessed 1 April 2019). DOI: https://doi.org/10.5772/8077
  19. Mihi A., Míguez H. Origin of light-harvesting enhancement in colloidal-photonic-crystal-based dye-sensitized solar cells. J. Phys. Chem. B, 2005, vol. 109, iss. 33, pp. 15968–76. DOI: https://doi.org/10.1021/jp051828g
  20. Furutsu K., Yamada Y. Diffusion approximation for adissipative random medium and the applications. Phys.Rev. E, 1994, vol. 50, iss. 5, pp. 3634–3640. DOI: https://doi.org/10.1103/PhysRevE.50.3634
  21. Zimnyakov D. A., Oh J.-T., Sinichkin Yu. P., Trifonov V. A., Gurianov E. V. Polarization-sensitive speckle spectroscopy of scattering media beyond the diffusion limit. J. Opt. Soc. Am. A, 2004, vol. 21, iss. 59, pp. 59–70. DOI: https://doi.org/10.1364/JOSAA.21.000059
  22. Born M., Wolf E. Principles of Optics. 7th ed. Cambridge, Cambridge University Press. 1999. 987 p.